Enantioselective copper-catalyzed allylic alkylations were performed on allylic bromides with a protectedhydroxyl or amine functional group using several Grignard reagents and Taniaphos L1 as a ligand. Theterminal olefin moiety in the products was transformed into various functional groups without racemization,providing facile access to a variety of versatile bifunctional chiral building blocks.