About: Branching Ratios in Activated Systems

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Attributs	Valeurs
type	work Article
Is Part Of	http://hub.abes.fr/acs/periodical/jpcafh/1997/volume_101/issue_1/w
Subject	Article
Title	Branching Ratios in Activated Systems
has manifestation of work	http://hub.abes.fr/acs/periodical/jpcafh/1997/volume_101/issue_1/101021jp961665j/m/print http://hub.abes.fr/acs/periodical/jpcafh/1997/volume_101/issue_1/101021jp961665j/m/web
related by	http://hub.abes.fr/acs/periodical/jpcafh/1997/volume_101/issue_1/101021jp961665j/authorship/4 http://hub.abes.fr/acs/periodical/jpcafh/1997/volume_101/issue_1/101021jp961665j/authorship/1 http://hub.abes.fr/acs/periodical/jpcafh/1997/volume_101/issue_1/101021jp961665j/authorship/3 http://hub.abes.fr/acs/periodical/jpcafh/1997/volume_101/issue_1/101021jp961665j/authorship/2
Author	Craig Stephen L. Brauman John I. Choo Bryan Zhong Meili
Abstract	Branching between reaction channels in activated systems is oftenobserved to vary with changes in thepotential energy surface asΔln(k1/k2) ∝Δ(Δ−Δ).RRKM calculations demonstrate that in many, butnot all, cases the log−linear relationship accurately describesbranching in nonthermal distributions of reactantswith energies well above the threshold for reaction. The origin ofthis relationship and conditions necessaryfor its validity can be understood in terms of quantum RRKtheory.
article type	research-article
is part of this journal	The Journal of Physical Chemistry A

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